Beilstein J. Nanotechnol.2019,10, 1217–1227, doi:10.3762/bjnano.10.121
). Moreover, following our recent achievements in the field of steam- and oxygen-free dehydrogenationcatalysis using CTFs as metal-free catalysts, the new samples with highest N contents have been scrutinized in the process to provide additional insights to their complex structure–activity relationship
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Keywords: covalent triazine frameworks; CO2 adsorption; CO2/N2 selectivity; dehydrogenationcatalysis; ionothermal conditions; Introduction
Recent years have witnessed an increasing interest in carbon-based nanomaterials as functional devices for energy-related applications [1]. Their unique properties
stability) as metal-free catalysts in gas-phase processes. Our recent achievements in the use of highly porous and N-rich carbon nanomaterials as metal-free catalysts for the steam- and oxygen-free dehydrogenationcatalysis (DDH) of ethylbenzene (EB) to styrene (ST) have shown unique outcomes in terms of
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Scheme 1:
Idealized ionothermal synthesis of CTF1–5 from 1,4-dicyanobenzene (p-DCB, I), 4,4′-dicyanobiphenyl ...